Journal of Industrial and Engineering Chemistry, Vol.67, 301-311, November, 2018
Fe0/C-bentonite alginate beads and oyster shell fixed-bed column combined process to continuously remove N-acetyl-p-aminophenol in persulfate system
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In this study, the ion-gelation method was applied to fabricate novel Fe.carbon.bentonite.alginate beads (Fe0/C-BABs). Fe0/C-BABs could effectively control Fe release during persulfate (PS) activation in Nacetyl- p-aminophenol (APAP) oxidation. A novel two-stage approach that combined Fe0/C-BABs and an oyster-shell-filled bed (OSFB) column was developed to address the low pH and high Fe concentration of the effluent of the traditional PS process. The application of the Fe0/C-BABs and OSFB column regulated pH levels and Fe release during the advanced oxidation of APAP. The characteristics of Fe0/C BABs were also investigated through scanning electron microscopy, energy dispersive spectrometry, and Fourier transform infrared spectroscopy. The long-term operation performance of Fe0/C-BABs in a continuous fixed-bed reactor under simultaneous PS and APAP feeding was also evaluated. The effects of initial PS concentration, pH, fixed-bed weight, in-flow rate, and dissolved oxygen (DO) were investigated. Under selected conditions, 86.3% efficiency was achieved during the first stage of APAP degradation (effluent pH of 3.05, Fe contents: 106.25 mg L-1). Water quality improved after the effluent was passed through the OSFB column (effluent pH of 6.32, Fe contents: 21.43 mg L-1). Moreover, this study analyzed the free radicals and intermediates produced during APAP degradation to identify the possible routes of APAP degradation.
Keywords:Fe0/C-bentonite alginate beads;Oyster shell;N-Acetyl-ρ-aminophenol;Fixed-bed column reactor;Persulfate
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